Monday, February 27, 2012

Ultrashort pulse

In optics, an ultrashort beating of ablaze is an electromagnetic beating whose time continuance is of the adjustment of a femtosecond (10 − 15 second). Such pulses accept a broadband optical spectrum, and can be created by mode-locked oscillators. They are frequently referred to as ultrafast events.

They are characterized by a top aiguille acuteness (or added correctly, irradiance) that usually leads to nonlinear interactions in assorted materials, including air. These processes are advised in the acreage of nonlinear optics.

In the specialized literature, "ultrashort" refers to the femtosecond (fs) to picosecond (ps) range, although such pulses no best authority the almanac for the beeline pulses artificially generated. Indeed, beating durations on the attosecond time calibration accept been reported.

The 1999 Nobel Prize in Chemistry was awarded to Ahmed H. Zewail for application ultrashort pulses to beam actinic reactions on the timescales they action on, aperture up the acreage of femtochemistry.

Definition

calculations, a circuitous acreage E(t) is defined. Formally, it is authentic as the analytic arresting agnate to the absolute field.

The axial angular abundance ω0 is usually absolutely accounting in the circuitous field, which may be afar as an acuteness action I(t) and a appearance action ψ(t):

E(t) = \sqrt{I(t)}e^{i\omega_0t}e^{i\psi(t)}

The announcement of the circuitous electric acreage in the abundance area is acquired from the Fourier transform of E(t):

E(\omega) = \mathcal{F}(E(t))

Because of the attendance of the e^{i\omega_0t} term, E(ω) is centered about ω0, and it is a accepted convenance to accredit to E(ω-ω0) by autograph just E(ω), which we will do in the blow of this article.

Just as in the time domain, an acuteness and a appearance action can be authentic in the abundance domain:

E(\omega) = \sqrt{S(\omega)}e^{i\phi(\omega)}

The abundance S(ω) is the ashen body (or simply, the spectrum) of the pulse, and φ(ω) is the ashen phase. Example of ashen appearance functions cover the case area φ(ω) is a constant, in which case the beating is alleged a bandwidth-limited pulse, or area φ(ω) is a boxlike function, in which case the beating is alleged a chirped beating because of the attendance of an direct abundance sweep. Such a call may be acquired as a beating propagates through abstracts (like glass) and is due to their dispersion. It after-effects in a banausic adorning of the pulse.

The acuteness functions I(t) and S(ω) actuate the time continuance and ashen bandwidth of the pulse. As declared by the ambiguity principle, their artefact (sometimes alleged the time-bandwidth product) has a lower bound. This minimum amount depends on the analogue acclimated for the continuance and on the appearance of the pulse. For a accustomed spectrum, the minimum time-bandwidth product, and accordingly the beeline pulse, is acquired by a transform-limited pulse, i.e., for a connected ashen appearance φ(ω). High ethics of the time-bandwidth product, on the added hand, announce a added circuitous pulse.

Pulse shape control

Although optical accessories aswell acclimated for connected light, like axle expanders and spatial filters, may be acclimated for ultrashort pulses, several optical accessories accept been accurately advised for ultrashort pulses. One of them is the beating compressor1, a accessory that can be acclimated to ascendancy the ashen appearance of ultrashort pulses. It is composed of a arrangement of prisms, or gratings. When appropriately adapted it can adapt the ashen appearance φ(ω) of the ascribe beating so that the achievement beating is a bandwidth-limited beating with the beeline accessible duration. A beating shaper can be acclimated to accomplish added complicated alterations on both the appearance and the amplitude of ultrashort pulses.

To accurately ascendancy the pulse, a abounding assuming of the beating ashen appearance is a have to in adjustment to get assertive beating ashen appearance (such as Transform-Limited). Then, a Spatial ablaze modulator can be acclimated in the 4f even to ascendancy the pulse. Multiphoton Intrapulse Interference Appearance Browse (MIIPS) is a address based on this concept. Through the appearance browse of the spatial ablaze modulator, MIIPS can not alone characterize but aswell dispense the ultrashort beating to get the bare beating appearance at ambition atom (such as transform-limited beating for optimized aiguille power, and added specific beating shapes). This address appearance with abounding arrangement and ascendancy of the ultrashort pulse, with no affective parts, and simple optical setup.

Measurement techniques

Several techniques are accessible to admeasurement ultrashort optical pulses:

acuteness autocorrelation: gives the beating amplitude if a accurate beating appearance is assumed.

ashen interferometry (SI): a beeline address that can be acclimated if a pre-characterized advertence beating is available. Gives the acuteness and phase. The algorithm that extracts the acuteness and appearance from the SI arresting is direct.

Ashen appearance interferometry for absolute electric-field about-face (SPIDER): a nonlinear self-referencing address based on ashen shearing interferometry. The adjustment is agnate to SI, except that the advertence beating is a spectrally confused replica of itself, acceptance one to access the ashen acuteness and appearance of the delving beating via a absolute FFT clarification accepted agnate to SI, but which requires affiliation of the appearance extracted from the interferogram to access the delving beating phase.

Frequency-resolved optical gating (FROG): a nonlinear address that yields the acuteness and appearance of a pulse. It's just a spectrally bound autocorrelation. The algorithm that extracts the acuteness and appearance from a FROG trace is iterative.

Grating-eliminated common ascertainment of ultrafast adventure laser ablaze e-fields (GRENOUILLE), a simplified adaptation of FROG.

Methods of anecdotic and authoritative the ultrashort optical pulses:

MIIPS Multiphoton Intrapulse Interference Appearance Scan, a adjustment to characterize and dispense the ultrashort pulse.


Wave packet propagation in nonisotropic media

To partially reiterate the altercation above, the boring capricious envelope approximation (SVEA) of the electric acreage of a beachcomber with axial beachcomber agent \textbf{K}_0 and axial abundance ω0 of the pulse, is accustomed by:

\textbf{E} ( \textbf{x} , t) = \textbf{ A } ( \textbf{x} , t) \exp ( i \textbf{K}_0 \textbf{x} - i \omega_0 t )

We accede the advancement for the SVEA of the electric acreage in a constant dispersive nonistropic medium. Assuming the beating is breeding in the administration of the z-axis, it can be apparent that the envelope \textbf{A} for one of the a lot of accepted of cases, namely a biaxial crystal, is absolute by the PDE2:

\frac{\partial \textbf{A} }{\partial z } = ~-~ \beta_1 \frac{\partial \textbf{A} }{\partial t} ~-~ \frac{i}{2} \beta_2 \frac{\partial^2 \textbf{A} }{\partial t^2} ~+~ \frac{1}{6} \beta_3 \frac{\partial^3 \textbf{A} }{\partial t^3} ~+~ \gamma_x \frac{\partial \textbf{A} }{\partial x} ~+~ \gamma_y \frac{\partial \textbf{A} }{\partial y}

~~~~~~~~~~~ ~+~ i \gamma_{tx} \frac{\partial^2 \textbf{A} }{\partial t \partial x} ~+~ i \gamma_{ty} \frac{\partial^2 \textbf{A} }{\partial t \partial y} ~-~ \frac{i}{2} \gamma_{xx} \frac{\partial^2 \textbf{A} }{ \partial x^2} ~-~ \frac{i}{2} \gamma_{yy} \frac{\partial^2 \textbf{A} }{ \partial y^2} ~+~ i \gamma_{xy} \frac{\partial^2 \textbf{A} }{ \partial x \partial y} + \ldots

where the coefficients contains diffraction and burning furnishings which accept been bent analytically with computer algebra and absolute numerically to aural third adjustment for both isotropic and non-istropic media, accurate in the near-field and far-field. β1 is the changed of the accumulation acceleration projection. The appellation in β2 is the accumulation acceleration burning (GVD) or second-order dispersion; it increases the beating continuance and chirps the beating as it propagates through the medium. The appellation in β3 is a third-order burning appellation that can added admission the beating duration, even if β2 vanishes. The agreement in γx and γy call the walk-off of the pulse; the accessory \gamma_x ~ (\gamma_y ) is the arrangement of the basic of the accumulation acceleration x ~ (y) and the assemblage agent in the administration of advancement of the beating (z-axis). The agreement in γxx and γyy call diffraction of the optical beachcomber packet in the admonition erect to the arbor of propagation. The agreement in γtx and γty absolute alloyed derivatives in time and amplitude circle the beachcomber packet about the y and x axes, respectively, admission the banausic amplitude of the beachcomber packet (in accession to the admission due to the GVD), admission the burning in the x and y directions, respectively, and admission the call (in accession to that due to β2) if the closing and/or γxx and γyy are nonvanishing. The appellation γxy rotates the beachcomber packet in the x − y plane. Oddly enough, because of ahead abridged expansions, this circling of the beating was not accomplished until the backward 1990s but it has been experimentally confirmed.3 To third order, the RHS of the aloft blueprint is begin to accept these added agreement for the uniaxial clear case4:

\ldots ~+~ \frac{1}{3} \gamma_{t x x } \frac{\partial^3 \textbf{A} }{ \partial x^2 \partial t} ~+~ \frac{1}{3} \gamma_{t y y } \frac{\partial^3 \textbf{A} }{ \partial y^2 \partial t} ~+~ \frac{1}{3} \gamma_{t t x } \frac{\partial^3 \textbf{A} }{ \partial t^2 \partial x} + \ldots

The aboriginal and added agreement are amenable for the curvature of the breeding foreground of the pulse. These terms, including the appellation in β3 are present in an isotropic average and annual for the all-around apparent of a breeding foreground basic from a point source. The appellation γtxx can be bidding in agreement of the basis of refraction, the abundance ω and derivatives thereof and the appellation γttx aswell distorts the beating but in a appearance that reverses the roles of t and x (see advertence of Trippenbach, Scott and Band for details). So far, the analysis herein is linear, but nonlinear dispersive agreement are all-over to nature. Studies involving an added nonlinear appellation γnl | A | 2A accept apparent that such agreement accept a abstruse aftereffect on beachcomber packet, including amidst added things, a self-steepening of the beachcomber packet.5 The non-linear aspects eventually advance to optical solitons.

Despite getting rather common, the SVEA is not appropriate to codify a simple beachcomber blueprint anecdotic the advancement of optical pulses. In fact, as apparent in,6 even a actual accepted anatomy of the electromagnetic added adjustment beachcomber blueprint can be factorized into directional components, accouterment admission to a individual aboriginal adjustment beachcomber blueprint for the acreage itself, rather than an envelope. This requires alone an acceptance that the acreage change is apathetic on the calibration of a wavelength, and does not bind the bandwidth of the beating at all—as approved vividly by.7

Applications

Micro-machining

Femtochemistry

Medical imaging: Ultrashort laser pulses are acclimated in multiphoton fluorescence microscopes

Terahertz (T-rays) bearing and detection.

abundance comb